To calculate the compositions of glasses with predicted hydrogen permeability, it is necessary to apply criteria that determine the structure of a substance, such as a silicate modulus, a connectivity factor, and a structure filling factor, as well as a glass comparison factor for a connectivity factor. A graphical method for optimizing the numerical values ??of these criteria has been developed. The compositions of glasses that are promising for the manufacture of hydrogen microballoons are presented. Tab. 2, ill. 1, bibliography: 22 titles.